Tale of a Gutsy Ninja - The Jiraiya Ninja Chronicles
Having become genin, Jiraiya, Tsunade, and Orochimaru are assigned to the future Third Hokage's platoon. Watching Sarutobi's space/time ninjutsu, Jiraiya becomes absorbed into learning it. One day, Jiraiya loses his way and stumbles upon Myouboku Mountain. There he meets the Great Toad Sage who predicted his arrival. See the origins of the Toad Sage Jiraiya!
Aired 24/09/2009EP 128 - Tale of a Gutsy Ninja - The Jiraiya Ninja Chronicles

Naruto: Shippuden
Naruto: Shippuuden is the continuation of the original animated TV series Naruto. The story revolves around an older and slightly more matured Uzumaki Naruto and his quest to save his friend Uchiha Sasuke from the grips of the snake-like Shinobi, Orochimaru. After 2 and a half years Naruto finally returns to his village of Konoha, and sets about putting his ambitions to work, though it will not be easy, as he has amassed a few (more dangerous) enemies, in the likes of the shinobi organization; Akatsuki.
(Source: Anime News Network)